My favorite DiMarzio humbuckers will be the Breed neck and the Breed bridge. They sound pretty warm, fat, smooth, big, not very modern sounding and not very vintage sounding.
Without a doubt for me it is the 36th Anniversary PAF. Love that pickup, I did help beta test it so I may be a little skewed...
I really just love what Steve Blucher did on that pickup. Of course it is vintage sounding but that is what I like. It is very articulate and it is the closest I have found to the pickups in my '64 345.
I have a Strat that has 3 of the HS-2's that will never leave that Strat.
If you haven't tried it already, try wiring your bridge HS-2 as a single-coil, that how Eric Johnson always ran his HS-2's, it sounds killer. The pickup gets a tad hotter when split.